Gespeichert in:
Titel: | Spectroscopic investigation of charge-transfer processes and polarisation pulse shaping in the visible spectral range |
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Weiterer Titel: | Spektroskopische Untersuchung von Ladungstransferprozessen und Polarisationspulsformung im sichtbaren Spektralbereich |
Von: |
von Tatjana Quast
|
Person: |
Quast, Tatjana
1982- Verfasser aut |
Hauptverfasser: | |
Format: | Abschlussarbeit Buch |
Sprache: | Englisch |
Veröffentlicht: |
2012
|
Schlagworte: | |
Online-Zugang: | https://nbn-resolving.org/urn:nbn:de:bvb:20-opus-74265 http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=025671741&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
Beschreibung: | Zsfassung in dt. und engl. Sprache. - Online erschienen 2013 |
Beschreibung: | VIII, 141 S. Ill., graph. Darst. |
Internformat
MARC
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245 | 1 | 0 | |a Spectroscopic investigation of charge-transfer processes and polarisation pulse shaping in the visible spectral range |c von Tatjana Quast |
246 | 1 | 3 | |a Spektroskopische Untersuchung von Ladungstransferprozessen und Polarisationspulsformung im sichtbaren Spektralbereich |
264 | 1 | |c 2012 | |
300 | |a VIII, 141 S. |b Ill., graph. Darst. | ||
336 | |b txt |2 rdacontent | ||
337 | |b n |2 rdamedia | ||
338 | |b nc |2 rdacarrier | ||
500 | |a Zsfassung in dt. und engl. Sprache. - Online erschienen 2013 | ||
502 | |a Würzburg, Univ., Diss., 2012 | ||
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Datensatz im Suchindex
DE-BY-OTHR_katkey | 5064160 |
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DE-BY-TUM_katkey | 1907225 |
DE-BY-UBR_katkey | 5064160 |
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adam_text | IMAGE 1
CONTENTS
LIST O F PUBLICATIONS III
1 MOTIVATION 1
2 THEORETICAL BACKGROUND 5
2.1 MATHEMATICAL DESCRIPTION OF FEMTOSECOND LASER PULSES 6 2.1.1 TIME
AND FREQUENCY REPRESENTATIONS OF THE ELECTRIC FIELD 6 2.1.2 SPATIAL
PROPAGATION OF LASER PULSES 9
2.1.3 EXTENSION TO ARBITRARILY POLARISED LASER PULSES 12 2.1.4 SPATIAL
BEAM PROFILE 13
2.2 NONLINEAR OPTICAL PROCESSES 16
2.2.1 FREQUENCY-SPACE DESCRIPTION OF THE NONLINEAR POLARISATION 16 2.2.2
SECOND-ORDER SUSCEPTIBILITY 16
2.2.3 THIRD-ORDER SUSCEPTIBILITY 17
2.3 POTENTIAL ENERGY SURFACES AND TRANSIENT ABSORPTION SPECTROSCOPY 22
2.3.1 ELECTRONIC TRANSITIONS IN MOLECULES 22
2.3.2 TRANSIENT ABSORPTION SPECTROSCOPY 25
2.4 QUANTUM CONTROL WITH SHAPED LASER PULSES 28
2.4.1 QUANTUM CONTROL SCHEMES 28
2.4.2 ADAPTIVE QUANTUM CONTROL 31
2.5 FOURIER-TRANSFORM PULSE SHAPING 34
3 CHARGE-TRANSFER DYNAMICS IN VARIOUS MOLECULAR STRUCTURES 39 3.1
NEUTRAL ORGANIC MIXED-VALENCE COMPOUNDS 42
3.2 THEORETICAL DESCRIPTION OF CHARGE-TRANSFER PROCESSES 45 3.2.1 MARCUS
THEORY 45
3.2.2 MARCUS-HUSH AND MULLIKEN-HUSH THEORY 48
3.2.3 THE BIXON-JORTNER MODEL 49
3.3 THE TRANSIENT SPECTROMETER 52
3.3.1 1KHZ SHOT-TO-SHOT TRANSIENT SPECTROMETER 52
3.3.2 HIGH REPETITION RATE TRANSIENT SPECTROMETER 54
V
HTTP://D-NB.INFO/1034061208
IMAGE 2
VI
3.4 GLOBAL ANALYSIS OF TRANSIENT ABSORPTION SPECTRA 58
4 NEUTRAL LOW-BAND-GAP MIXED-VALENCE POLYMER 63
4.1 PREVIOUS RESEARCH ON MONOMERIC TARA-PCTM CHARGE-TRANSFER COMPOUNDS
65
4.2 TARA-PCTM POLYMER 69
4.3 TRANSIENT ABSORPTION SPECTROSCOPY OF TARA-PCTM COMPOUNDS 71 4.3.1
TRANSIENT ABSORPTION DATA FOR P AND M 71
4.3.2 GLOBAL ANALYSIS OF THE KINETICS 77
4.3.3 INTERPRETATION OF THE TRANSIENT ABSORPTION DATA 83 4.4 OUTLOOK:
OLIGOMERS AND EXCITON-EXCITON ANNIHILATION 87
5 DONOR-SUBSTITUTED TRUXENONES 91
5.1 TARA-SUBSTITUTED TRUXENONES 92
5.2 ULTRAFAST SPECTROSCOPY OF TRUXENONES 95
5.2.1 TRANSIENT ABSORPTION SPECTROSCOPY 95
5.2.2 TRANSIENT ANISOTROPY 101
5.2.3 GLOBAL ANALYSIS OF THE TRANSIENT ABSORPTION DATA . . . . 103 5.2.4
INTERPRETATION OF THE TRUXENONE DATA 109
5.3 CONCLUSION TRUXENONES 114
6 METALLO-SUPRAMOLECULAR POLYELECTROLYTE 117
6.1 PROPERTIES OF MEPES 119
6.1.1 GENERAL PROPERTIES 119
6.1.2 PROPERTIES OF FE-MEPE-LL AND FE-L2 121
6.2 TRANSIENT ABSORPTION SPECTROSCOPY OF MEPES 124
6.3 GLOBAL ANALYSIS OF THE MEPE DATA 127
6.4 INTERPRETATION OF THE MEPE DATA 130
6.5 OUTLOOK: FURTHER RESEARCH ON MEPE 132
6.5.1 FUTURE MEPE EXPERIMENTS 132
6.5.2 IMPROVEMENT OF DATA QUALITY 133
7 BROADBAND VISIBLE POLARISATION PULSE SHAPING 135
7.1 PULSE-SHAPER SETUP 140
7.2 PULSE CHARACTERISATION 143
7.2.1 FREQUENCY-RESOLVED OPTICAL GATING 143
7.2.2 SPECTRAL INTERFEROMETRY 148
7.2.3 JONES-MATRIX CALCULUS 157
7.3 GENERATION AND CHARACTERISATION OF POLARISATION-SHAPED LASER PULSES
160
IMAGE 3
CONTENTS VII
7.3.1 PULSE COMPRESSION 160
7.3.2 CORRECTION FACTOR FOR POLARISATION-DEPENDENT DETECTION EFFICIENCY
163
7.3.3 DETERMINATION OF THE REFERENCE PHASE 167
7.3.4 JONES-MATRIX MEASUREMENT 170
7.3.5 RELATIVE PHASE DQSI 172
7.3.6 ERROR CALCULATION 174
7.3.7 COMPARISON OF FTSI AND DQSI 177
7.4 CONCLUSIONS ON POLARISATION PULSE SHAPING 187
8 SUMMARY 191
ZUSAMMENFASSUNG 195
ACKNOWLEDGEMENTS 235
LEBENSLAUF 239
ERKLARUNG 241
|
any_adam_object | 1 |
author | Quast, Tatjana 1982- |
author_GND | (DE-588)1030021910 |
author_facet | Quast, Tatjana 1982- |
author_role | aut |
author_sort | Quast, Tatjana 1982- |
author_variant | t q tq |
building | Verbundindex |
bvnumber | BV040690995 |
collection | ebook |
ctrlnum | (OCoLC)826601548 (DE-599)BVBBV040690995 |
format | Thesis Book |
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genre_facet | Hochschulschrift |
id | DE-604.BV040690995 |
illustrated | Illustrated |
indexdate | 2024-12-20T16:23:27Z |
institution | BVB |
language | English |
oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-025671741 |
oclc_num | 826601548 |
open_access_boolean | 1 |
owner | DE-384 DE-473 DE-BY-UBG DE-703 DE-1051 DE-824 DE-29 DE-12 DE-91 DE-BY-TUM DE-19 DE-BY-UBM DE-1049 DE-92 DE-739 DE-898 DE-BY-UBR DE-355 DE-BY-UBR DE-706 DE-20 DE-1102 |
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physical | VIII, 141 S. Ill., graph. Darst. |
psigel | ebook |
publishDate | 2012 |
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record_format | marc |
spellingShingle | Quast, Tatjana 1982- Spectroscopic investigation of charge-transfer processes and polarisation pulse shaping in the visible spectral range Polarisiertes Licht (DE-588)4278185-1 gnd Ladungstransfer (DE-588)4307016-4 gnd Optische Spektroskopie (DE-588)4043680-9 gnd |
subject_GND | (DE-588)4278185-1 (DE-588)4307016-4 (DE-588)4043680-9 (DE-588)4113937-9 |
title | Spectroscopic investigation of charge-transfer processes and polarisation pulse shaping in the visible spectral range |
title_alt | Spektroskopische Untersuchung von Ladungstransferprozessen und Polarisationspulsformung im sichtbaren Spektralbereich |
title_auth | Spectroscopic investigation of charge-transfer processes and polarisation pulse shaping in the visible spectral range |
title_exact_search | Spectroscopic investigation of charge-transfer processes and polarisation pulse shaping in the visible spectral range |
title_full | Spectroscopic investigation of charge-transfer processes and polarisation pulse shaping in the visible spectral range von Tatjana Quast |
title_fullStr | Spectroscopic investigation of charge-transfer processes and polarisation pulse shaping in the visible spectral range von Tatjana Quast |
title_full_unstemmed | Spectroscopic investigation of charge-transfer processes and polarisation pulse shaping in the visible spectral range von Tatjana Quast |
title_short | Spectroscopic investigation of charge-transfer processes and polarisation pulse shaping in the visible spectral range |
title_sort | spectroscopic investigation of charge transfer processes and polarisation pulse shaping in the visible spectral range |
topic | Polarisiertes Licht (DE-588)4278185-1 gnd Ladungstransfer (DE-588)4307016-4 gnd Optische Spektroskopie (DE-588)4043680-9 gnd |
topic_facet | Polarisiertes Licht Ladungstransfer Optische Spektroskopie Hochschulschrift |
url | https://nbn-resolving.org/urn:nbn:de:bvb:20-opus-74265 http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=025671741&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
work_keys_str_mv | AT quasttatjana spectroscopicinvestigationofchargetransferprocessesandpolarisationpulseshapinginthevisiblespectralrange AT quasttatjana spektroskopischeuntersuchungvonladungstransferprozessenundpolarisationspulsformungimsichtbarenspektralbereich |